Над альбомом работал бразильский композитор Эйтор Перейра (Angry Birds в кино, Хэйвен, Простые сложности), а его релиз состоялся 26 июля 2011 года. На саундтрек попало 36 композиций общей длительностью более часа. Подборка является компиляцией оригинальной музыки. Выпуском пластинки занимался лейбл Madison Gate Records.
CD 1
| 1 | Race to the VillageHeitor Pereira | 02:22 |  |
| 2 | Gargamel's Smurf PlanHeitor Pereira | 02:00 | |
| 3 | Blue Moon PredictionsHeitor Pereira | 00:57 | |
| 4 | It's InvisibleHeitor Pereira | 01:17 | |
| 5 | The VortexHeitor Pereira | 03:35 | |
| 6 | Where the Smurfs Are We?Heitor Pereira | 01:28 | |
| 7 | Clumsy Gets In the BoxHeitor Pereira | 02:00 | |
| 8 | Sweet Folicular AmbrosiaHeitor Pereira | 02:43 | |
| 9 | Clumsy's Out Of the BoxHeitor Pereira | 04:37 | |
| 10 | Is Everyone In This Realm Insane?Heitor Pereira | 01:06 | |
| 11 | Arrival At AnjelouHeitor Pereira | 03:05 | |
| 12 | Emerging Through the SmokeHeitor Pereira | 00:46 | |
| 13 | The Genius That Is GargamelHeitor Pereira | 02:24 | |
| 14 | You Can Be Anything You Want to BeHeitor Pereira | 01:07 | |
| 15 | Chamber PotHeitor Pereira | 02:03 | |
| 16 | Find That Star GazerHeitor Pereira | 00:53 | |
| 17 | FAO SmurfsHeitor Pereira | 00:47 | |
| 18 | Get Out of My Suck a Ma JigHeitor Pereira | 03:16 | |
| 19 | Inspired or SafeHeitor Pereira | 01:23 | |
| 20 | Another Smurfless NightHeitor Pereira | 01:12 | |
| 21 | You're a Good PapaHeitor Pereira | 01:46 | |
| 22 | Behold My Glorious ArmyHeitor Pereira | 00:40 | |
| 23 | The Perfect Time to Smurf the Blue …Heitor Pereira | 02:38 | |
| 24 | Baby's First PictureHeitor Pereira | 01:46 | |
| 25 | The History of SmurfsHeitor Pereira | 01:41 | |
| 26 | Cautiously ExcitedHeitor Pereira | 01:58 | |
| 27 | Aaah, It's Gargamel!Heitor Pereira | 01:21 | |
| 28 | We RideHeitor Pereira | 01:12 | |
| 29 | I So Smurfin' Love YouHeitor Pereira | 01:31 | |
| 30 | My Smurf Magic MachineHeitor Pereira | 01:19 | |
| 31 | Blue Moon IncantationHeitor Pereira | 01:08 | |
| 32 | Enjoy the Ride PapaHeitor Pereira | 01:08 | |
| 33 | Smurfs Stand UpHeitor Pereira | 01:40 | |
| 34 | The Awesome Power of MeHeitor Pereira | 03:17 | |
| 35 | Clumsy's Got ItHeitor Pereira | 00:54 | |
| 36 | I Smurf YouHeitor Pereira | 04:16 | |
